Discovery of BAZ2A bromodomain ligands.

نویسندگان

  • Dimitrios Spiliotopoulos
  • Eike-Christian Wamhoff
  • Graziano Lolli
  • Christoph Rademacher
  • Amedeo Caflisch
چکیده

The bromodomain adjacent to zinc finger domain protein 2A (BAZ2A) is implicated in aggressive prostate cancer. The BAZ2A bromodomain is a challenging target because of the shallow pocket of its natural ligand, the acetylated side chain of lysine. Here, we report the successful screening of a library of nearly 1500 small molecules by high-throughput docking and force field-based binding-energy evaluation. For seven of the 20 molecules selected in silico, evidence of binding to the BAZ2A bromodomain is provided by ligand-observed NMR spectroscopy. Two of these compounds show a favorable ligand efficiency of 0.42 kcal/mol per non-hydrogen atom in a competition-binding assay. The crystal structures of the BAZ2A bromodomain in complex with four fragment hits validate the predicted binding modes. The binding modes of compounds 1 and 3 are compatible with ligand growing for optimization of affinity for BAZ2A and selectivity against the close homologue BAZ2B.

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عنوان ژورنال:
  • European journal of medicinal chemistry

دوره 139  شماره 

صفحات  -

تاریخ انتشار 2017